The nearest pickup point for the hop on hop off bus is on Marylebone Road just east of the junction with Baker Street. The Big Bus stops there, and I very much suspect that the Original Tour will stop there as well, since it's very near - sigh - Madame Tussaud's.
The walk from Marylebone station to the stops mentioned above shouldn't take much more than ten minutes. Fares for the hop on hop off buses are around £25 for adults.
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